Muon spin rotation and relaxation studies have been performed on a "111" family of iron-based superconductors NaFe_1-xNi_xAs. Static magnetic order was characterized by obtaining the temperature and doping dependences of the local ordered magnetic moment size and the volume fraction of the magnetically ordered regions. For x = 0 and 0.4 %, a transition to a nearly-homogeneous long range magnetically ordered state is observed, while for higher x than 0.4 % magnetic order becomes more disordered and is completely suppressed for x = 1.5 %. The magnetic volume fraction continuously decreases with increasing x. The combination of magnetic and superconducting volumes implies that a spatially-overlapping coexistence of magnetism and superconductivity spans a large region of the T-x phase diagram for NaFe_1-xNi_xAs . A strong reduction of both the ordered moment size and the volume fraction is observed below the superconducting T_C for x = 0.6, 1.0, and 1.3 %, in contrast to other iron pnictides in which one of these two parameters exhibits a reduction below TC, but not both. The suppression of magnetic order is further enhanced with increased Ni doping, leading to a reentrant non-magnetic state below T_C for x = 1.3 %. The reentrant behavior indicates an interplay between antiferromagnetism and superconductivity involving competition for the same electrons. These observations are consistent with the sign-changing s-wave superconducting state, which is expected to appear on the verge of microscopic coexistence and phase separation with magnetism. We also present a universal linear relationship between the local ordered moment size and the antiferromagnetic ordering temperature TN across a variety of iron-based superconductors. We argue that this linear relationship is consistent with an itinerant-electron approach, in which Fermi surface nesting drives antiferromagnetic ordering.

Disentangling superconducting and magnetic orders in NaFe_1-xNi_xAs using muon spin rotation / Cheung, S.C., Zurab, G., Frandsen, B.A., Zizhou, G., Kohtaro, Y., Almeida, D.E., Onuorah, I.J., Bonfa', P., Eduardo, M., Weiyi, W., Tam, D.W., Song, Y.u., Chongde, C., Yipeng, C., Hallas, A.M., Wilson, M.N., Munsie, T.J.S., Graeme, L., Bijuan, C., Guangyang, D., et al.. - In: PHYSICAL REVIEW. B. - ISSN 2469-9950. - 97:22(2018), p. 224508. [10.1103/PhysRevB.97.224508]

Disentangling superconducting and magnetic orders in NaFe_1-xNi_xAs using muon spin rotation

ONUORAH, IFEANYI JOHN;Pietro Bonfa;Roberto De Renzi;
2018-01-01

Abstract

Muon spin rotation and relaxation studies have been performed on a "111" family of iron-based superconductors NaFe_1-xNi_xAs. Static magnetic order was characterized by obtaining the temperature and doping dependences of the local ordered magnetic moment size and the volume fraction of the magnetically ordered regions. For x = 0 and 0.4 %, a transition to a nearly-homogeneous long range magnetically ordered state is observed, while for higher x than 0.4 % magnetic order becomes more disordered and is completely suppressed for x = 1.5 %. The magnetic volume fraction continuously decreases with increasing x. The combination of magnetic and superconducting volumes implies that a spatially-overlapping coexistence of magnetism and superconductivity spans a large region of the T-x phase diagram for NaFe_1-xNi_xAs . A strong reduction of both the ordered moment size and the volume fraction is observed below the superconducting T_C for x = 0.6, 1.0, and 1.3 %, in contrast to other iron pnictides in which one of these two parameters exhibits a reduction below TC, but not both. The suppression of magnetic order is further enhanced with increased Ni doping, leading to a reentrant non-magnetic state below T_C for x = 1.3 %. The reentrant behavior indicates an interplay between antiferromagnetism and superconductivity involving competition for the same electrons. These observations are consistent with the sign-changing s-wave superconducting state, which is expected to appear on the verge of microscopic coexistence and phase separation with magnetism. We also present a universal linear relationship between the local ordered moment size and the antiferromagnetic ordering temperature TN across a variety of iron-based superconductors. We argue that this linear relationship is consistent with an itinerant-electron approach, in which Fermi surface nesting drives antiferromagnetic ordering.
2018
Disentangling superconducting and magnetic orders in NaFe_1-xNi_xAs using muon spin rotation / Cheung, S.C., Zurab, G., Frandsen, B.A., Zizhou, G., Kohtaro, Y., Almeida, D.E., Onuorah, I.J., Bonfa', P., Eduardo, M., Weiyi, W., Tam, D.W., Song, Y.u., Chongde, C., Yipeng, C., Hallas, A.M., Wilson, M.N., Munsie, T.J.S., Graeme, L., Bijuan, C., Guangyang, D., et al.. - In: PHYSICAL REVIEW. B. - ISSN 2469-9950. - 97:22(2018), p. 224508. [10.1103/PhysRevB.97.224508]
File in questo prodotto:
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11381/2840314
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 12
  • ???jsp.display-item.citation.isi??? 11
social impact